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Influence of conversion material morphology on electrochemistry studied with operando X-ray tomography and diffraction


Villevieille, Claire; Ebner, Martin; Gómez-Cámer, Juan Luis; Marone, Federica; Novák, Petr; Wood, Vanessa (2015). Influence of conversion material morphology on electrochemistry studied with operando X-ray tomography and diffraction. Advanced Materials, 27(10):1676-1681.

Abstract

X-ray diffraction and X-ray tomography are performed on intermetallic particles undergoing lithiation in a porous electrode. Differences between ensemble phase evolution and that at a single-particle level are explored. It is found that all particles evidence core-shell lithiation; however, particles with internal porosity are more mechanically robust and exhibit less fracture.

Abstract

X-ray diffraction and X-ray tomography are performed on intermetallic particles undergoing lithiation in a porous electrode. Differences between ensemble phase evolution and that at a single-particle level are explored. It is found that all particles evidence core-shell lithiation; however, particles with internal porosity are more mechanically robust and exhibit less fracture.

Citations

9 citations in Web of Science®
8 citations in Scopus®
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Additional indexing

Item Type:Journal Article, refereed, further contribution
Communities & Collections:04 Faculty of Medicine > Institute of Biomedical Engineering
Dewey Decimal Classification:170 Ethics
610 Medicine & health
Language:English
Date:2015
Deposited On:08 Feb 2016 14:22
Last Modified:05 Apr 2016 20:00
Publisher:Wiley-Blackwell Publishing, Inc.
ISSN:0935-9648
Publisher DOI:https://doi.org/10.1002/adma.201403792
PubMed ID:25619158

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