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Extended Corannulenes: Aromatic Bowl/Sheet Hybridization


Dutta, Amit K; Linden, Anthony; Zoppi, Laura; Baldridge, Kim K; Siegel, Jay S (2015). Extended Corannulenes: Aromatic Bowl/Sheet Hybridization. Angewandte Chemie Internationale Edition, 54(37):10792-10796.

Abstract

Among sheet/sheet polynuclear aromatic hydrocarbon (PAH) hybrids, a buckybowl–graphene hybrid has been used as a model to explore the effects of physical properties of PAHs with distinct planar and bowl regions. Activation of a C(Ar)¢F bond was used to synthesize this corannulene/graphenic hybrid. Photophysical and voltammetric studies together with high-level computations revealed curvature and extended p-effects on the properties of these materials.

Abstract

Among sheet/sheet polynuclear aromatic hydrocarbon (PAH) hybrids, a buckybowl–graphene hybrid has been used as a model to explore the effects of physical properties of PAHs with distinct planar and bowl regions. Activation of a C(Ar)¢F bond was used to synthesize this corannulene/graphenic hybrid. Photophysical and voltammetric studies together with high-level computations revealed curvature and extended p-effects on the properties of these materials.

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Additional indexing

Item Type:Journal Article, refereed, original work
Communities & Collections:07 Faculty of Science > Department of Chemistry
Dewey Decimal Classification:540 Chemistry
Uncontrolled Keywords:buckybowl–graphene hybrids · fused-ring systems · polyaromatic hydrocarbons · structure–activity relationships
Language:English
Date:2015
Deposited On:12 Nov 2015 09:13
Last Modified:16 Dec 2016 11:37
Publisher:Wiley-VCH Verlag
ISSN:1433-7851
Publisher DOI:https://doi.org/10.1002/anie.201503553

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