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The microscopic structure of charge density waves in underdoped YBa$_2$Cu$_3$O$_{6.54}$ revealed by X-ray diffraction


Forgan, E M; Blackburn, E; Holmes, A T; Briffa, A K R; Chang, J; Bouchenoire, L; Brown, S D; Liang, Ruixing; Bonn, D; Hardy, W N; Christensen, N B; Zimmermann, M V; Hücker, M; Hayden, S M (2015). The microscopic structure of charge density waves in underdoped YBa$_2$Cu$_3$O$_{6.54}$ revealed by X-ray diffraction. Nature Communications, 6:10064.

Abstract

Charge density wave (CDW) order appears throughout the underdoped high-temperature cuprate superconductors, but the underlying symmetry breaking and the origin of the CDW remain unclear. We use X-ray diffraction to determine the microscopic structure of the CDWs in an archetypical cuprate YBa$_2$Cu$_3$O$_{6.54}$ at its superconducting transition temperature ~60 K. We find that the CDWs in this material break the mirror symmetry of the CuO$_2$ bilayers. The ionic displacements in the CDWs have two components, which are perpendicular and parallel to the CuO$_2$ planes, and are out of phase with each other. The planar oxygen atoms have the largest displacements, perpendicular to the CuO$_2$ planes. Our results allow many electronic properties of the underdoped cuprates to be understood. For instance, the CDWs will lead to local variations in the electronic structure, giving an explicit explanation of density-wave states with broken symmetry observed in scanning tunnelling microscopy and soft X-ray measurements.

Abstract

Charge density wave (CDW) order appears throughout the underdoped high-temperature cuprate superconductors, but the underlying symmetry breaking and the origin of the CDW remain unclear. We use X-ray diffraction to determine the microscopic structure of the CDWs in an archetypical cuprate YBa$_2$Cu$_3$O$_{6.54}$ at its superconducting transition temperature ~60 K. We find that the CDWs in this material break the mirror symmetry of the CuO$_2$ bilayers. The ionic displacements in the CDWs have two components, which are perpendicular and parallel to the CuO$_2$ planes, and are out of phase with each other. The planar oxygen atoms have the largest displacements, perpendicular to the CuO$_2$ planes. Our results allow many electronic properties of the underdoped cuprates to be understood. For instance, the CDWs will lead to local variations in the electronic structure, giving an explicit explanation of density-wave states with broken symmetry observed in scanning tunnelling microscopy and soft X-ray measurements.

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Additional indexing

Item Type:Journal Article, refereed, original work
Communities & Collections:07 Faculty of Science > Physics Institute
Dewey Decimal Classification:530 Physics
Language:English
Date:2015
Deposited On:25 Jan 2016 14:41
Last Modified:07 Aug 2017 17:08
Publisher:Nature Publishing Group
ISSN:2041-1723
Free access at:PubMed ID. An embargo period may apply.
Publisher DOI:https://doi.org/10.1038/ncomms10064
PubMed ID:26648114

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