Publication: Sulfur-Treatment Passivates Bulk Defects in Sb2Se3 Photocathodes for Water Splitting
Sulfur-Treatment Passivates Bulk Defects in Sb2Se3 Photocathodes for Water Splitting
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Prabhakar, R. R., Moehl, T., Friedrich, D., Kunst, M., Shukla, S., Adeleye, D., Damle, V. H., Siol, S., Cui, W., Gouda, L., Suh, J., Tischler, Y. R., van de Krol, R., & Tilley, S. D. (2022). Sulfur-Treatment Passivates Bulk Defects in Sb2Se3 Photocathodes for Water Splitting. Advanced Functional Materials, 32(25), 2112184. https://doi.org/10.1002/adfm.202112184
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Sb2Se3 has emerged as an important photoelectrochemical (PEC) and photovoltaic (PV) material due to its rapid rise in photoconversion efficiencies. However, Sb2Se3 has a complex defect chemistry, which reduces the maximum photovoltage. Thus, it is important to understand these defects and develop defect passivation strategies in Sb2Se3. A comprehensive investigation of the charge carrier dynamics of Sb2Se3 and the influence of sulfur treatment on its optoelectronic properties is performed using time-resolved microwave conductivity (TR
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Prabhakar, R. R., Moehl, T., Friedrich, D., Kunst, M., Shukla, S., Adeleye, D., Damle, V. H., Siol, S., Cui, W., Gouda, L., Suh, J., Tischler, Y. R., van de Krol, R., & Tilley, S. D. (2022). Sulfur-Treatment Passivates Bulk Defects in Sb2Se3 Photocathodes for Water Splitting. Advanced Functional Materials, 32(25), 2112184. https://doi.org/10.1002/adfm.202112184