Publication: Mechanism of Photocatalytic Hydrogen Generation by a Polypyridyl-Based Cobalt Catalyst in Aqueous Solution
Mechanism of Photocatalytic Hydrogen Generation by a Polypyridyl-Based Cobalt Catalyst in Aqueous Solution
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Rodenberg, A., Orazietti, M., Probst, B., Bachmann, C., Alberto, R., Baldridge, K. K., & Hamm, P. (2015). Mechanism of Photocatalytic Hydrogen Generation by a Polypyridyl-Based Cobalt Catalyst in Aqueous Solution. Inorganic Chemistry, 54(2), 646–657. https://doi.org/10.1021/ic502591a
Abstract
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The mechanism of photocatalytic hydrogen production was studied with a three-component system consisting of fac-Re(py)(CO)(3)bipy (py = pyridine, bipy = 2,2'-bipyridine) as photosensitizer, Co(TPY-OH)(OH2) (TPY-OH = 2-bis(2-pyridyl)(hydroxy)methyl-6-pyridylpyridine), a polypyridyl-based cobalt complex, as water reduction catalyst (WRC), and triethanolamine (TEOA) as sacrificial electron donor in aqueous solution. A detailed mechanistic picture is provided, which covers all processes from excited state quenching on the time
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- Rodenberg, Alexander
- Orazietti, Margherita
- Probst, Benjamin
- Bachmann, Cyril
- Baldridge, Kim K
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Rodenberg, A., Orazietti, M., Probst, B., Bachmann, C., Alberto, R., Baldridge, K. K., & Hamm, P. (2015). Mechanism of Photocatalytic Hydrogen Generation by a Polypyridyl-Based Cobalt Catalyst in Aqueous Solution. Inorganic Chemistry, 54(2), 646–657. https://doi.org/10.1021/ic502591a
