Publication: Ultrafast Vibrational Energy Transfer in Catalytic Monolayers at Solid–Liquid Interfaces
Ultrafast Vibrational Energy Transfer in Catalytic Monolayers at Solid–Liquid Interfaces
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Kraack, J. P., Frei, A., Alberto, R., & Hamm, P. (2017). Ultrafast Vibrational Energy Transfer in Catalytic Monolayers at Solid–Liquid Interfaces. Journal of Physical Chemistry Letters, 8(11), 2489–2495. https://doi.org/10.1021/acs.jpclett.7b01034
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We investigate the ultrafast vibrational dynamics of monolayers from adsorbed rhenium–carbonyl CO2-reduction catalysts on a semiconductor surface (indium–tin-oxide (ITO)) with ultrafast two-dimensional attenuated total reflection infrared (2D ATR IR) spectroscopy. The complexes are partially equipped with isotope-labeled (13C) carbonyl ligands to generate two spectroscopically distinguishable forms of the molecules. Ultrafast vibrational energy transfer between the molecules is observed via the temporal evolution of cross-peaks betwee
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- Kraack, Jan Philip
- Frei, Angelo
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Kraack, J. P., Frei, A., Alberto, R., & Hamm, P. (2017). Ultrafast Vibrational Energy Transfer in Catalytic Monolayers at Solid–Liquid Interfaces. Journal of Physical Chemistry Letters, 8(11), 2489–2495. https://doi.org/10.1021/acs.jpclett.7b01034
