Publication: Ascorbate as an electron relay between an irreversible electron donor and Ru(ii) or Re(i) photosensitizers
Ascorbate as an electron relay between an irreversible electron donor and Ru(ii) or Re(i) photosensitizers
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Bachmann, C., Probst, B., Guttentag, M., & Alberto, R. (2014). Ascorbate as an electron relay between an irreversible electron donor and Ru(ii) or Re(i) photosensitizers. Chemical Communications, 50, 6737–6739. https://doi.org/10.1039/c4cc01500b
Abstract
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Ascorbate acts as a reversible electron shuttle between tris(2-carboxyethyl) phosphine (TCEP) and ReI or RuII photosensitizers. Oxidized ascorbate is recycled up to 50 times by the TCEP → TCEP[double bond, length as m-dash]O redox process which enables 30 000 TONs per WRC in photocatalytic hydrogen production, thus exceeding the performance with pure ascorbate by far.
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- Bachmann, Cyril
- Probst, Benjamin
- Guttentag, Miguel
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Bachmann, C., Probst, B., Guttentag, M., & Alberto, R. (2014). Ascorbate as an electron relay between an irreversible electron donor and Ru(ii) or Re(i) photosensitizers. Chemical Communications, 50, 6737–6739. https://doi.org/10.1039/c4cc01500b