Publication: 3d–4f {CoII3Ln(OR)4} Cubanes as Bio-Inspired Water Oxidation Catalysts
3d–4f {CoII3Ln(OR)4} Cubanes as Bio-Inspired Water Oxidation Catalysts
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Evangelisti, F., Moré, R., Hodel, F., Luber, S., & Patzke, G. R. (2015). 3d–4f {CoII3Ln(OR)4} Cubanes as Bio-Inspired Water Oxidation Catalysts. Journal of the American Chemical Society, 137(34), 11076–11084. https://doi.org/10.1021/jacs.5b05831
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Although the {CaMn4O5} oxygen evolving complex (OEC) of photosystem II is a major paradigm for water oxidation catalyst (WOC) development, the comprehensive translation of its key features into active molecular WOCs remains challenging. The [CoII3Ln(hmp)4(OAc)5H2O] ({CoII3Ln(OR)4}; Ln = Ho–Yb, hmp = 2-(hydroxymethyl)pyridine) cubane WOC series is introduced as a new springboard to address crucial design parameters, ranging from nuclearity and redox-inactive promoters to operational stability and ligand exchange properties. The {CoII3L
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- Evangelisti, Fabio
- Moré, René
- Hodel, Florian
- Luber, Sandra
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Evangelisti, F., Moré, R., Hodel, F., Luber, S., & Patzke, G. R. (2015). 3d–4f {CoII3Ln(OR)4} Cubanes as Bio-Inspired Water Oxidation Catalysts. Journal of the American Chemical Society, 137(34), 11076–11084. https://doi.org/10.1021/jacs.5b05831