Publication: Synthesis and Molecular Structure of 99Tc Corroles
Synthesis and Molecular Structure of 99Tc Corroles
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Einrem, R. F., Braband, H., Fox, T., Vazquez-Lima, H., Alberto, R., & Ghosh, A. (2016). Synthesis and Molecular Structure of 99Tc Corroles. Chemistry, 22, 18747–18751. https://doi.org/10.1002/chem.201605015
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The first 99Tc corroles have been synthesized and fully characterized. A single-crystal X-ray structure of a 99TcO triarylcorrole revealed nearly identical geometry parameters as the corresponding ReO structure. A significant spectral shift between the Soret maxima of TcO (410–413 nm) and ReO (438–441 nm) corroles was observed and, based on two-component spin–orbit ZORA TDDFT calculations, ascribed to relativistic effects in the Re case. The syntheses reported herein potentially pave the way toward 99mTc-porphyrinoid-based radiopharma
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- Einrem, Rune F
- Fox, Thomas
- Vazquez-Lima, Hugo
- Ghosh, Abhik
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Einrem, R. F., Braband, H., Fox, T., Vazquez-Lima, H., Alberto, R., & Ghosh, A. (2016). Synthesis and Molecular Structure of 99Tc Corroles. Chemistry, 22, 18747–18751. https://doi.org/10.1002/chem.201605015