Publication: Nickel-Catalyzed Enantioselective Electrochemical Reductive Cross-Coupling of Aryl Aziridines with Alkenyl Bromides
Nickel-Catalyzed Enantioselective Electrochemical Reductive Cross-Coupling of Aryl Aziridines with Alkenyl Bromides
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Hu, X., Cheng-Sánchez, I., Cuesta-Galisteo, S., & Nevado, C. (2023). Nickel-Catalyzed Enantioselective Electrochemical Reductive Cross-Coupling of Aryl Aziridines with Alkenyl Bromides. Journal of the American Chemical Society, 145(11), 6270–6279. https://doi.org/10.1021/jacs.2c12869
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An electrochemically driven nickel-catalyzed enantioselective reductive cross-coupling of aryl aziridines with alkenyl bromides has been developed, affording enantioenriched β-aryl homoallylic amines with excellent E-selectivity. This electroreductive strategy proceeds in the absence of heterogeneous metal reductants and sacrificial anodes by employing constant current electrolysis in an undivided cell with triethylamine as a terminal reductant. The reaction features mild conditions, remarkable stereocontrol, broad substrate scope, an
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- Hu, Xia
- Cheng-Sánchez, Iván
- Cuesta-Galisteo, Sergio
- Nevado, Cristina
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Hu, X., Cheng-Sánchez, I., Cuesta-Galisteo, S., & Nevado, C. (2023). Nickel-Catalyzed Enantioselective Electrochemical Reductive Cross-Coupling of Aryl Aziridines with Alkenyl Bromides. Journal of the American Chemical Society, 145(11), 6270–6279. https://doi.org/10.1021/jacs.2c12869
