Publication: The Furan Shuffling Hypothesis: A Biogenetic Proposal for Eremophilane Sesquiterpenoids
The Furan Shuffling Hypothesis: A Biogenetic Proposal for Eremophilane Sesquiterpenoids
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Lardon, N., Liffert, R., Linden, A., & Gademann, K. (2019). The Furan Shuffling Hypothesis: A Biogenetic Proposal for Eremophilane Sesquiterpenoids. Angewandte Chemie Internationale Edition, 58(21), 7004–7007. https://doi.org/10.1002/anie.201901898
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Based on the structural similarities of the recently isolated eremophilane‐type sesquiterpenoids microsphaeropsisin B and C and the iso‐eremophilane periconianone C, a revised biogenetic hypothesis for C8–C11‐connected iso‐eremophilanes is presented and corroborated by strong experimental evidence. The first enantioselective total syntheses of microsphaeropsisin B and C were achieved starting from a known intermediate, whose synthesis was elaborated previously in the total synthesis of periconianone A, and in a total of 15 steps start
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- Lardon, Nicolas
- Liffert, Raphael
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Lardon, N., Liffert, R., Linden, A., & Gademann, K. (2019). The Furan Shuffling Hypothesis: A Biogenetic Proposal for Eremophilane Sesquiterpenoids. Angewandte Chemie Internationale Edition, 58(21), 7004–7007. https://doi.org/10.1002/anie.201901898
