Publication: Understanding the Dynamics of Molecular Water Oxidation Catalysts with Liquid-Phase Transmission Electron Microscopy: The Case of Vitamin B12
Understanding the Dynamics of Molecular Water Oxidation Catalysts with Liquid-Phase Transmission Electron Microscopy: The Case of Vitamin B12
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Abdi, Z., Balaghi, S. E., Sologubenko, A. S., Willinger, M.-G., Vandichel, M., Shen, J.-R., Allakhverdiev, S. I., Patzke, G. R., & Najafpour, M. M. (2021). Understanding the Dynamics of Molecular Water Oxidation Catalysts with Liquid-Phase Transmission Electron Microscopy: The Case of Vitamin B12. ACS Sustainable Chemistry & Engineering, 9(28), 9494–9505. https://doi.org/10.1021/acssuschemeng.1c03539
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Cobalt compounds are intensely explored as efficient catalysts for the oxygen evolution reaction (OER). Since vitamin B12 is a soluble cobalt compound with high enzymatic activity, evaluating its OER activity is of relevance for biomimetic catalyst research. In this work, the temporal evolution of a homogenous vitamin B12 catalyst in the early stages of OER was investigated by an advanced combination of in situ electrochemical liquid transmission electron microscopy (EC-LTEM), in situ UV–vis spectroelectrochemistry, and extended X-ray
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- Abdi, Zahra
- Balaghi, S Esmael
- Sologubenko, Alla S
- Willinger, Marc-Georg
- Vandichel, Matthias
- Shen, Jian-Ren
- Allakhverdiev, Suleyman I
- Najafpour, Mohammad Mahdi
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Abdi, Z., Balaghi, S. E., Sologubenko, A. S., Willinger, M.-G., Vandichel, M., Shen, J.-R., Allakhverdiev, S. I., Patzke, G. R., & Najafpour, M. M. (2021). Understanding the Dynamics of Molecular Water Oxidation Catalysts with Liquid-Phase Transmission Electron Microscopy: The Case of Vitamin B12. ACS Sustainable Chemistry & Engineering, 9(28), 9494–9505. https://doi.org/10.1021/acssuschemeng.1c03539
