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Revealing the role of electrons and phonons in the ultrafast recovery of charge density wave correlations in $1T−TiSe_2$


Monney, C; Puppin, M; Nicholson, C W; Hoesch, M; Chapman, R. T; Springate, E; Berger, H; Magrez, A; Cacho, C; Ernstorfer, R; Wolf, M (2016). Revealing the role of electrons and phonons in the ultrafast recovery of charge density wave correlations in $1T−TiSe_2$. Physical Review B, 94(16):165165.

Abstract

Using time- and angle-resolved photoemission spectroscopy with selective near- and midinfrared photon excitations, we investigate the femtosecond dynamics of the charge density wave (CDW) phase in $1T−TiSe_2$ as well as the dynamics of CDW fluctuations at 240 K. In the CDW phase, we observe the coherent oscillation of the CDW amplitude mode. At 240 K, we single out an ultrafast component in the recovery of the CDW correlations, which we explain as the manifestation of electron-hole correlations. Our momentum-resolved study of femtosecond electron dynamics supports a mechanism for the CDW phase resulting from the cooperation between the interband Coulomb interaction, the mechanism of excitonic insulator phase formation, and electron-phonon coupling.

Abstract

Using time- and angle-resolved photoemission spectroscopy with selective near- and midinfrared photon excitations, we investigate the femtosecond dynamics of the charge density wave (CDW) phase in $1T−TiSe_2$ as well as the dynamics of CDW fluctuations at 240 K. In the CDW phase, we observe the coherent oscillation of the CDW amplitude mode. At 240 K, we single out an ultrafast component in the recovery of the CDW correlations, which we explain as the manifestation of electron-hole correlations. Our momentum-resolved study of femtosecond electron dynamics supports a mechanism for the CDW phase resulting from the cooperation between the interband Coulomb interaction, the mechanism of excitonic insulator phase formation, and electron-phonon coupling.

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Additional indexing

Item Type:Journal Article, refereed, original work
Communities & Collections:07 Faculty of Science > Physics Institute
Dewey Decimal Classification:530 Physics
Scopus Subject Areas:Physical Sciences > Electronic, Optical and Magnetic Materials
Physical Sciences > Condensed Matter Physics
Language:English
Date:2016
Deposited On:11 Jan 2017 18:02
Last Modified:30 Jul 2020 23:51
Publisher:American Physical Society
ISSN:2469-9950
OA Status:Hybrid
Publisher DOI:https://doi.org/10.1103/PhysRevB.94.165165
Project Information:
  • : FunderSNSF
  • : Grant IDPZ00P2_154867
  • : Project TitleTime- and angle-resolved photoemission spectroscopy on correlated materials

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