Publication: Light-Induced H2 Evolution with a Macrocyclic Cobalt Diketo-Pyrphyrin as a Proton-Reducing Catalyst
Light-Induced H2 Evolution with a Macrocyclic Cobalt Diketo-Pyrphyrin as a Proton-Reducing Catalyst
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Joliat-Wick, E., Weder, N., Klose, D., Bachmann, C., Spingler, B., Probst, B., & Alberto, R. (2018). Light-Induced H2 Evolution with a Macrocyclic Cobalt Diketo-Pyrphyrin as a Proton-Reducing Catalyst. Inorganic Chemistry, 57, 1651–1655. https://doi.org/10.1021/acs.inorgchem.7b02992
Abstract
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Cobalt complexes are well-known catalysts for photocatalytic proton reduction in water. Macrocyclic tetrapyridyl ligands (pyrphyrins) and their CoII complexes emerged in this context as a highly efficient class of H2 evolution catalysts. On the basis of this framework, a new macrocyclic CoII complex consisting of two keto-bridged bipyridyl units (Co diketo-pyrphyrin) is presented. The complex is synthesized along a convenient route, is well soluble in water, and shows high activity as a water reduction catalyst (WRC). In an aqueous sy
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- Joliat-Wick, Evelyne
- Weder, Nicola
- Klose, Daniel
- Bachmann, Cyril
- Probst, Benjamin
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Joliat-Wick, E., Weder, N., Klose, D., Bachmann, C., Spingler, B., Probst, B., & Alberto, R. (2018). Light-Induced H2 Evolution with a Macrocyclic Cobalt Diketo-Pyrphyrin as a Proton-Reducing Catalyst. Inorganic Chemistry, 57, 1651–1655. https://doi.org/10.1021/acs.inorgchem.7b02992