Publication: Electrocatalytic Ammonia Oxidation with a Tailored Molecular Catalyst Heterogenized via Surface Host–Guest Complexation
Electrocatalytic Ammonia Oxidation with a Tailored Molecular Catalyst Heterogenized via Surface Host–Guest Complexation
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Roithmeyer, H., Sévery, L., Moehl, T., Spingler, B., Blacque, O., Fox, T., Iannuzzi, M., & Tilley, S. D. (2024). Electrocatalytic Ammonia Oxidation with a Tailored Molecular Catalyst Heterogenized via Surface Host–Guest Complexation. Journal of the American Chemical Society, 146(1), 430–436. https://doi.org/10.1021/jacs.3c09725
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Macrocyclic host mols. bound to electrode surfaces enable the complexation of catalytically active guests for mol. heterogeneous catalysis. The authors present a surface-anchored host-guest complex with the ability to electrochem. oxidize NH3 in both organic and aqueous solutions With an adamantyl motif as the binding group on the backbone of the mol. catalyst Ru(bpy-NMe2)(tpada)(Cl) (1) (bpy-NMe2 is 4,4′-bis(dimethylamino)-2,2′-bipyridyl, tpada is 4′-(adamantan-1-yl)-2,2′:6′,2′′-terpyridine), high binding constants with β-cycl
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- Roithmeyer, Helena
- Sévery, Laurent
- Moehl, Thomas
- Blacque, Olivier
- Fox, Thomas
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Roithmeyer, H., Sévery, L., Moehl, T., Spingler, B., Blacque, O., Fox, T., Iannuzzi, M., & Tilley, S. D. (2024). Electrocatalytic Ammonia Oxidation with a Tailored Molecular Catalyst Heterogenized via Surface Host–Guest Complexation. Journal of the American Chemical Society, 146(1), 430–436. https://doi.org/10.1021/jacs.3c09725
