Publication: Electronic Coupling of Molecular Complexes to Au Electrodes Mediated via Host–Guest Interactions
Electronic Coupling of Molecular Complexes to Au Electrodes Mediated via Host–Guest Interactions
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Tuncay, I., Chang Chien, T.-C., Keller, F., Roithmeyer, H., Sévery, L., Blacque, O., Iannuzzi, M., Delley, M. F., & Tilley, S. D. (2025). Electronic Coupling of Molecular Complexes to Au Electrodes Mediated via Host–Guest Interactions. Journal of the American Chemical Society, 148(1), 330–339. https://doi.org/10.1021/jacs.5c12957
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Immobilization of molecular catalysts onto electrode surfaces using host-guest (HG) interactions enables the facile regeneration of electrodes following catalyst degradation. Beyond this practical aspect, the architecture also offers a unique way to study the electronic coupling of molecules to the electrode through a nominally insulating linker. Here, we employ surface-enhanced infrared absorption spectroscopy (SEIRAS) to characterize the binding and electronic coupling of Au-bound HG complexes. Distinct spectral features and binding
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Tuncay, I., Chang Chien, T.-C., Keller, F., Roithmeyer, H., Sévery, L., Blacque, O., Iannuzzi, M., Delley, M. F., & Tilley, S. D. (2025). Electronic Coupling of Molecular Complexes to Au Electrodes Mediated via Host–Guest Interactions. Journal of the American Chemical Society, 148(1), 330–339. https://doi.org/10.1021/jacs.5c12957
