Publication: CO2 to CO: Photo‐ and electrocatalytic conversion based on Re(I) Bis‐Arene Frameworks: synergisms between catalytic subunits
CO2 to CO: Photo‐ and electrocatalytic conversion based on Re(I) Bis‐Arene Frameworks: synergisms between catalytic subunits
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Hernández‐Valdés, D., Fernández-Terán, R., Probst, B., Spingler, B., & Alberto, R. (2020). CO2 to CO: Photo‐ and electrocatalytic conversion based on Re(I) Bis‐Arene Frameworks: synergisms between catalytic subunits. Helvetica Chimica Acta, 103(10), e2000147. https://doi.org/10.1002/hlca.202000147
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Reduction of CO2 to CO and H2O is a two electron/two proton process. For this process, multinuclear complexes offer advantages by concentrating reduction equivalents more efficiently than mononuclear systems. We present novel complexes with [Re(η6‐C6H6)2]+ as scaffold conjugated to one or two catalytically active [Ru(dmbpy)(CO)2Cl2] subunits (dmbpy=5,5′‐dimethyl‐2,2′‐bipyridine). The [Re(η6‐C6H6)2]+ scaffold was chosen due to its very high photo‐ and chemical stability, as well as the multiple degrees of freedom it offers for any conj
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- Hernández‐Valdés, Daniel
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Hernández‐Valdés, D., Fernández-Terán, R., Probst, B., Spingler, B., & Alberto, R. (2020). CO2 to CO: Photo‐ and electrocatalytic conversion based on Re(I) Bis‐Arene Frameworks: synergisms between catalytic subunits. Helvetica Chimica Acta, 103(10), e2000147. https://doi.org/10.1002/hlca.202000147
